Next, the solution mixture is sufficiently stirred using a dispersing machine such as a ball mill, thereby obtaining a slurry. Next, the slurry is applied on the first main surface of the porous self-supporting film, for example, by a doctor blade method. At this time, while the solid electrolyte particles in the slurry hardly enter the pores of the porous self-supporting film, the solvent in the slurry enters the pores of the porous self-supporting film and reaches the second main surface. Since at least a portion of the polymeric material is dissolved in the slurry, the polymeric material also reaches the second main surface from the first main surface of the porous self-supporting film, and a coating is formed on at least a portion of the second main surface. Next, the coating is dried to remove the solvent, whereby it is possible to obtain a separator including a solid electrolyte layer containing the second binder and the first binder existing on the second main surface of the porous self-supporting film.